GUI means Graphical User Interface, so it's everything you're looking at. Like now, when you read this post you'll probably be reading it from a browser; this browser have a graphical user interface - it's everything you're looking at. As default, Python ships with Tkinter, so you could try out some GUI-programming right away, without installing new libraries.
From what you're saying you know, you should be able to make the famous guess-a-number-game. It requires you to have the basic understanding of modules and user I/O though.
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